DOI QR코드

DOI QR Code

High-Speed High-Resolution Terahertz Time-Domain Spectrometer

고속 고분해 테라헤르츠 시간영역 분광기

  • Kim, Young-Chan (Safety Metrology Center, Korea Research Institute of Standards and Science) ;
  • Kim, Ki-Bok (Safety Metrology Center, Korea Research Institute of Standards and Science) ;
  • Yee, Dae-Su (Safety Metrology Center, Korea Research Institute of Standards and Science) ;
  • Yi, Min-Woo (Dept. of Physics, Korea Advanced Institute of Science & Technology) ;
  • Ahn, Jae-Wook (Dept. of Physics, Korea Advanced Institute of Science & Technology)
  • 김영찬 (한국표준과학연구원 안전계측연구단) ;
  • 김기복 (한국표준과학연구원 안전계측연구단) ;
  • 이대수 (한국표준과학연구원 안전계측연구단) ;
  • 이민우 (한국과학기술원 물리학과) ;
  • 안재욱 (한국과학기술원 물리학과)
  • Published : 2008.10.25

Abstract

High-speed high-resolution terahertz time-domain spectroscopy (THz-TDS) is demonstrated using the asynchronous-opticalsampling (AOS) method. A time-domain signal with a 10-ns time window is rapidly acquired by using two femtosecond lasers with slightly different repetition frequencies to generate and detect a terahertz pulse wave, without a mechanical delay stage. The spectrum obtained by the fast Fourier transformation (FFT) of the time-domain waveform has a frequency resolution of 100 MHz. The time resolution of our spectrometer is measured using the cross-correlation method to be 278 fs. A transmission spectrum of water vapor is measured and the absorption lines are analyzed in the frequency range from 0.1 to 1.2 THz.

본 논문에서 비동시성 광샘플링(asynchronous optical sampling; AOS) 방식을 이용하는 고속 고분해 테라헤르츠 시간영역 분광(terahertz time domain spectroscopy; THz-TDS)을 시연한다. 모터로 구동되는 선형 스테이지를 사용하지 않고, 약간 다른 반복 주파수를 갖는 두 대의 펨토초 레이저를 각각 테라헤르츠파 발생과 검출에 사용하여 고속으로 10 ns의 시간축 상의 신호를 획득하고 fast Fourier transformation(FFT)을 통하여 100 MHz의 주파수 분해능을 갖는 고분해 분광을 구현한다. Cross-correlation 방법에 의해 시간 분해능은 278 fs으로 측정되었다. 또한, 본 분광기를 이용하여 수증기의 투과 스펙트럼을 측정하고 흡수선들을 분석하였다.

Keywords

References

  1. C. Sirtori, "Bridge for the terahertz gap," Nature, vol. 417, no. 6885, pp. 132-133, 2002 https://doi.org/10.1038/417132b
  2. K. Kawase, Y. Ogawa, Y. Watanabe, and H. Inoue, "Nondestructive terahertz imaging of illicit drugs using spectral fingerprints," Opt. Express, vol. 11, no. 20, pp. 2549-2554, 2003 https://doi.org/10.1364/OE.11.002549
  3. S. Nakajima, H. Hoshina, M. Yamashita, C. Otani, and N. Miyoshi, "Terahertz imaging diagnostics of cancer tissues with a chemometrics technique," Appl. Phys. Lett., vol. 90, no. 4, p. 041102, 2007 https://doi.org/10.1063/1.2433035
  4. P. A. Elzinga, R. J. Kneisler, F. E. Lytle, Y. Jiang, G. B. King, and N. M. Laurendeau, "Pump/probe method for fast analysis of visible spectral signatures utilizing asynchronous optical sampling," Appl. Opt., vol. 26, no. 19, pp. 4303-4309, 1987 https://doi.org/10.1364/AO.26.004303
  5. Y. Takagi and S. Adachi, "Subpicosecond optical sampling spectrometer using asynchronous tunable mode-locked lasers," Rev. Sci. Instrum., vol. 70, no. 5, pp. 2218-2224, 1999 https://doi.org/10.1063/1.1149740
  6. T. Yasui, E. Saneyoshi, and T. Araki, "Asynchronous optical sampling terahertz time-domain spectroscopy for ultrahigh spectral resolution and rapid data acquisition," Appl. Phys. Lett., vol. 87, no. 6, p. 061101, 2005 https://doi.org/10.1063/1.2008379
  7. C. Janke, M. Forst, M. Nagel, H. Kurz, and A. Bartels, "Asynchronous optical sampling for high-speed characterization of integrated resonant terahertz sensors," Opt. Lett., vol. 30, no. 11, pp. 1405-1407, 2005 https://doi.org/10.1364/OL.30.001405
  8. A. Bartels, R. Cerna, C. Kistner, A. Thoma, F. Hudert, C. Janke, and T. Dekorsy, "Ultrafast time-domain spectroscopy based on high-speed asynchronous optical sampling," Rev. Sci. Instrum., vol. 78, no. 3, p. 035107, 2007 https://doi.org/10.1063/1.2714048
  9. C. Kistner, A. Andre, T. Fischer, A. Thoma, C. Janke, A. Bartels, T. Gisler, G. Maret, and T. Dekorsy, "Hydration dynamics of oriented DNA films investigated by timedomain terahertz spectroscopy," Appl. Phys. Lett., vol. 90, no. 23, p. 233902, 2007 https://doi.org/10.1063/1.2743401
  10. P. R. Griffiths, Chemical Infrared Fourier Transform Spectroscopy (Wiley, New York, USA, 1975), pp. 89-91
  11. M. van Exter, Ch. Fattinger, and D. Grischkowsky, "Terahertz time-domain spectroscopy of water vapor," Opt. Lett., vol. 14, no. 20, pp. 1128-1130, 1989 https://doi.org/10.1364/OL.14.001128

Cited by

  1. Terahertz Spectroscopy: System and Sensitivity Considerations vol.1, pp.1, 2011, https://doi.org/10.1109/TTHZ.2011.2159877