Journal of Electrochemical Science and Technology

The Korean Electrochemical Society (한국전기화학회)
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Characterization of Anodized Al 1050 with Electrochemically Deposited Cu, Ni and Cu/Ni and Their Behavior in a Model Corrosive Medium

  • Girginov, Christian (Department of Physical Chemistry, University of Chemical Technology and Metallurgy) ;
  • Kozhukharov, Stephan (Laboratory for Advanced Materials Research, University of Chemical Technology and Metallurgy) ;
  • Tsanev, Alexander (Institute of General and Inorganic Chemistry, Bulgarian Academy of Sciences) ;
  • Dishliev, Angel (Department of Mathematics, University of Chemical Technology and Metallurgy)
  • Received : 2020.07.21
  • Accepted : 2020.10.06
  • Published : 2021.05.28
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Abstract

The specific benefits of the modified films formed on preliminary anodized aluminum, including the versatility of their potential applications impose the need for evaluation of the exploitation reliability of these films. In this aspect, the durability of Cu and Ni modified anodized aluminum oxide (AAO) films on the low-doped AA1050 alloy was assessed through extended exposure to a 3.5% NaCl model corrosive medium. The electrochemical measurements by means of electrochemical impedance spectroscopy (EIS) and potentiodynamic scanning (PDS) after 24 and 720 hours of exposure have revealed that the obtained films do not change their obvious barrier properties. In addition, supplemental analyses of the coatings were performed, in order to elucidate the impact of the AC-deposition of Cu and Ni inside the pores. The scanning electron microscopy (SEM) images have shown that the surface topology is not affected and resembles the typical surface of an etched metal. The subsequent energy dispersive X-ray spectroscopy (EDX) tests have revealed a predominance of Cu in the combined AAO-Cu/Ni layers, whereas additional X-ray photoelectron (XPS) analyses showed that both metals form oxides with different oxidation states due to alterations in the deposition conditions, promoted by the application of AC-polarization of the samples.

Keywords

Acknowledgement

The authors would like to express their gratitude to the Bulgarian National Scientific Fund for the financial support under contract No. KП-06-M 38/1 (2019).

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