Journal of the Korean Institute of Electrical and Electronic Material Engineers (한국전기전자재료학회논문지)

The Korean Institute of Electrical and Electronic Material Engineers (한국전기전자재료학회)
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Perspective on Ferroelectric Polymers Presenting Negative Longitudinal Piezoelectric Coefficient and Morphotropic Phase Boundary

강유전체 고분자의 음의 압전 물성 및 상공존경계(MPB)에 대한 고찰

  • Im, Sungbin (Division of Advanced Materials Engineering, Jeonbuk National University) ;
  • Bu, Sang Don (Department of Physics, Jeonbuk National University) ;
  • Jeong, Chang Kyu (Division of Advanced Materials Engineering, Jeonbuk National University)
  • 임성빈 (전북대학교 신소재공학부 전자재료공학전공) ;
  • 부상돈 (전북대학교 물리학과) ;
  • 정창규 (전북대학교 신소재공학부 전자재료공학전공)
  • Received : 2022.08.12
  • Accepted : 2022.08.24
  • Published : 2022.11.01
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Abstract

Morphotropic phase boundary (MPB), which is a special boundary that separates two or multiple different phases in the phase diagram of some ferroelectric ceramics, is an important concept in identifying physics that includes piezoelectric responses. MPB, which had not been discovered in organic materials until recently, was discovered in poly(vinylidene fluoride-co-trifluoroethylene (P(VDF-TrFE)), resulting from a molecular approach. The piezoelectric coefficient of P(VDF-TrFE) in this MPB region was achieved up to -63.5 pC N-1, which is about two times as large as the conventional value of -30 pC N-1 of P(VDF-TrFE). An order-disorder arrangement greatly affects the rise of the piezoelectric effect and the ferroelectric, paraelectric and relaxor ferroelectric of P(VDF-TrFE), so the arrangement and shape of the polymer chain is important. In this review, we investigate the origin of negative longitudinal piezoelectric coefficients of piezoelectric polymers, which is definitely opposite to those of common piezoelectric ceramics. In addition to the mainly discussed issue about MPB behaviors of ferroelectric polymers, we also introduce the consideration about polymer chirality resulting in relaxor ferroelectric properties. When the physics of ferroelectric polymers is unveiled, we can improve the piezoelectric and pyroelectric properties of ferroelectric polymers and contribute to the development of next-generation sensor, energy, transducer and actuator applications.

Keywords

Acknowledgement

본 연구는 2022년 과학기술정보통신부 재원으로 한국연구재단의 지원(2022R1A2C4002037, 2022R1A4A3032923)을 받아 수행된 결과입니다.

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