Let 𝚽 be a continuous, strictly increasing, subadditive, positive and concave function on (0, ∞) of critical lower type index $p^{-}_{\Phi}{\in}(0,1]$, and ${\rho}(t)=\frac{t^{-1}}{{\Phi}^{-1}(t^{-1})}$ for t ∈ (0, ∞). Let n ∈ ℕ, 𝛼 ∈ (0, min{2, n}), ${\gamma}{\in}[0,\,\frac{n}{{\alpha}})$, and $a^{\ast}:=-\frac{2^{\alpha}{\Gamma}((n+{\alpha})/4)^2}{{\Gamma}((n-{\alpha})/4)^2}$. For any a ∈ [a*, ∞), the fractional Schrödinger operator L𝛼 is defined by L𝛼 := (-∆)𝛼/2 + a|x|-𝛼. In this article, the authors first introduce the VMO-type space VMO𝛾,M𝜌,L𝛼 (ℝn) associated with L𝛼, and then characterize these spaces via some tent spaces. Moreover, the authors also show that, for any given $p^{-}_{\Phi}{\in}(\frac{n}{n+{\alpha}},\,1]$, VMO1,M𝜌,L𝛼 (ℝn) space is the predual space of the Orlicz-Hardy space H𝚽L𝛼 (ℝn) associated with L𝛼. These results generalize the known recent results by particularly taking 𝚽(t) = tp for any t ∈ (0, ∞) and $p{\in}(\frac{n}{n+{\alpha}},\,1]$.