• 제목/요약/키워드: Radiocesium Migration

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Temporal Change in Radiological Environments on Land after the Fukushima Daiichi Nuclear Power Plant Accident

  • Saito, Kimiaki;Mikami, Satoshi;Andoh, Masaki;Matsuda, Norihiro;Kinase, Sakae;Tsuda, Shuichi;Sato, Tetsuro;Seki, Akiyuki;Sanada, Yukihisa;Wainwright-Murakami, Haruko;Yoshimura, Kazuya;Takemiya, Hiroshi;Takahashi, Junko;Kato, Hiroaki;Onda, Yuichi
    • Journal of Radiation Protection and Research
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    • 제44권4호
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    • pp.128-148
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    • 2019
  • Massive environmental monitoring has been conducted continuously since the Fukushima Daiichi Nuclear Power accident in March of 2011 by different monitoring methods that have different features together with migration studies of radiocesium in diverse environments. These results have clarified the characteristics of radiological environments and their temporal change around the Fukushima site. At three months after the accident, multiple radionuclides including radiostrontium and plutonium were detected in many locations; and it was confirmed that radiocesium was most important from the viewpoint of long-term exposure. Radiation levels around the Fukushima site have decreased greatly over time. The decreasing trend was found to change variously according to local conditions. The air dose rates in environments related to human living have decreased faster than expected from radioactive decay by a factor of 2-3 on average; those in pure forest have decreased more closely to physical decay. The main causes of air dose rate reduction were judged to be radioactive decay, movement of radiocesium in vertical and horizontal directions, and decontamination. Land-use categories and human activities have significantly affected the reduction tendency. Difference in the air dose rate reduction trends can be explained qualitatively according to the knowledge obtained in radiocesium migration studies; whereas, the quantitative explanation for individual sites is an important future challenge. The ecological half-lives of air dose rates have been evaluated by several researchers, and a short-term half-life within 1 year was commonly observed in the studies. An empirical model for predicting air dose rate distribution was developed based on statistical analysis of an extensive car-borne survey dataset, which enabled the prediction with confidence intervals. Different types of contamination maps were integrated to better quantify the spatial data. The obtained data were used for extended studies such as for identifying the main reactor that caused the contamination of arbitrary regions and developing standard procedures for environmental measurement and sampling. Annual external exposure doses for residents who intended to return to their homes were estimated as within a few millisieverts. Different forms of environmental data and knowledge have been provided for wide spectrum of people. Diverse aspects of lessons learned from the Fukushima accident, including practical ones, must be passed on to future generations.

Sorption and Migration Studies of Fission Products for Ground Waste Disposal

  • Lee, Sang-Hoon;Chun, Kwan-Sik;Yoon, Young-Ku
    • Nuclear Engineering and Technology
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    • 제10권3호
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    • pp.153-163
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    • 1978
  • 부지주변 환경과 관련한 방사성 고체 폐기물의 지중처분 문제는, 비록 안전하고 경제적이라 할지라도, 대단히 중요하다. 지중처분을 위한 방사성 핵중(Sr-90, Cs-137)의 이동과 물의 이동에 관한 연구가 실험실과 야외에서 수행되었다. 방사성 핵종에 대한 토양의 친화력은 알칼리성 용액에서 더 강하고, 흡착은 시간에 대한 함수관계가 있음을 나타내었다. 방사성스트론티움과 세시움의 이동율은 3.73$\times$$10^{-3}$-10.9$\times$$^{-3}$cm/day로서, 물의 이동 속도 보다 훨씬 낮은 값을 나타내었으며, 이것은 아마도 높은 이온이온교환능에 기인되는 것이다. 확산에 기초를 둔 수학적인 모형에 의거 얻은 값과 측정 트리티움의 분포가 비교되었다. 지하에서의 물의 이동 현상을 규명하는데 삼중수를 추적자료로 이용할 수 있음을 암시하고 있다.

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Radiation Monitoring in the Residential Environment: Time Dependencies of Air Dose Rate and 137Cs Inventory

  • Yoshimura, Kazuya;Nakama, Shigeo;Fujiwara, Kenso
    • Journal of Radiation Protection and Research
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    • 제47권1호
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    • pp.30-38
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    • 2022
  • Background: Residential areas have some factors on the external exposure of residents, who usually spend a long time in these areas. Although various survey has been carried out by the government or the research institutions after the Fukushima Daiichi Nuclear Power Plant accident, the mechanism of radiocesium inventory in the terrestrial zone has not been cleared. To better evaluate the radiation environment, this study investigated the temporal changes in air dose rate and 137Cs inventories (Bq/m2) in residential areas and agricultural fields. Materials and Methods: Air dose rate and 137Cs inventories were investigated in residential areas located in an evacuation zone at 5-8 km from the Fukushima Daiichi Nuclear Power Plant. From December 2014 to September 2018, the air dose rate distribution was investigated through a walking survey (backpack survey), which was conducted by operators carrying a γ-ray detector on their backs. Additionally, from December 2014 to January 2021, the 137Cs inventories on paved and permeable grounds were also measured using a portable γ-ray detector. Results and Discussion: In the areas where decontamination was not performed, the air dose rate decreased faster in residential areas than in agricultural fields. Moreover, the 137Cs inventory on paved surfaces decreased with time owing to the horizontal wash-off, while the 137Cs inventory on permeable surfaces decreased dramatically owing to the decontamination activities. Conclusion: These findings suggest that the horizontal wash-off of 137Cs on paved surfaces facilitated the air dose rate decrease in residential areas to a greater extent compared with agricultural fields, in which the air dose rate decreased because of the vertical migration of 137Cs. Results of this study can explain the faster environmental restoration in a residential environment reported by previous studies.